# Silicon dioxide Silicon dioxide is a two-species network-former. Each Si sits at the centre of a tetrahedron of four O neighbours (Si-O ≈ 1.61 Å), and each O bridges two Si atoms. The reference here is α-quartz (trigonal *P*3₁21, *a* = 4.9134 Å, *c* = 5.4052 Å) tiled into an orthogonal **40 × 40 × 40 Å** supercell by `tricor.Supercell`. Instead of drawing pairwise bonds, each panel renders a translucent polyhedron around every Si whose four nearest O neighbours form a near-ideal tetrahedron (bond length within ±15 % of 1.61 Å, all six O-Si-O angles within ±25° of 109.47°). ## Overview All six regimes at an orthogonal 40 × 40 × 40 Å supercell, rotating in sync. Drag any panel to orbit manually. g(r) per regime overlaid on a single axis (most disordered curve at the bottom, most ordered at the top). The dropdown below the plot switches between the three species pairs in alphabetical order (`O-O`, `O-Si`, `Si-Si`); only `O-Si` is a real chemical bond, the other two peaks are lattice separations through a bridging atom. The Si-O peak at 1.61 Å sharpens monotonically up the ladder; the Si-Si and O-O second-shell peaks at 2.64 / 3.06 Å develop crystalline fine structure (split shells) only at LRO / NC. ## Reference crystal ```python from ase.io import read atoms_ref = read('structures/SiO2.cif') # 3 Si + 6 O ``` ## Supercell `tricor.Supercell` tiles the α-quartz primitive into a Cartesian 40 × 40 × 40 Å box. The algorithm seeds Voronoi cells, tiles the reference out to a sphere that covers the largest cell, rotates the tile per grain (identity rotation when ``grain_size=None``), and filters atoms by exact convex-hull membership against each Voronoi cell. Per-species atom counts are then pinned to the reference stoichiometry scaled by ``V_box / V_ref × relative_density`` so every regime has identical Si and O counts, and grain-boundary overlaps are culled at ``0.9 × hard_min``. ```python import tricor as tc # Only Si-O is a real chemical bond in SiO2. The second-shell # Si-Si (3.06 Å) and O-O (2.64 Å) peaks are lattice separations # through a bridging atom; ``from_atoms`` zeroes their coordination # targets automatically (``auto_filter_lattice_artifacts=True``), so # they install no bond springs. shell_target = tc.CoordinationShellTarget.from_atoms(atoms_ref, phi_num_bins=90) cell = tc.Supercell.from_atoms( atoms_ref, cell_dim_angstroms=(40, 40, 40), r_max=10, r_step=0.1, phi_num_bins=90, rng_seed=42, ) cell.generate(shell_target, grain_size=None) # liquid; see regime pages ``` ## Disorder regimes ```{toctree} :maxdepth: 1 liquid amorphous short_range_order medium_range_order long_range_order nanocrystalline ``` ## Preset summary | Regime | `num_steps` | `grain_size` (Å) | `bond_weight` | `angle_weight` | `repulsion_weight` | `hard_core_scale` | `nonbond_push_scale` | `displacement_sigma` | |---|---|---|---|---|---|---|---|---| | liquid | 120 | - | 0.50 | 0.0 | 1.5 | 1.05 | 0.60 | 0.010 | | amorphous | 250 | 12.0 | 1.55 | 1.25 | 1.25 | 0.81 | 0.70 | 0.012 | | short-range order | 250 | 15.0 | 1.65 | 1.35 | 1.30 | 0.82 | 0.72 | 0.010 | | medium-range order | 300 | 20.0 | 1.65 | 1.35 | 1.30 | 0.82 | 0.72 | 0.008 | | long-range order | 350 | 26.0 | 1.65 | 1.35 | 1.30 | 0.82 | 0.72 | 0.006 | | nanocrystalline | 400 | 35.0 | 1.65 | 1.35 | 1.30 | 0.82 | 0.72 | 0.003 | The liquid panel uses `angle_weight=0` so the random starting positions aren't pulled into tetrahedral coordination by the angle spring; every other regime keeps the angle spring on so SiO₄ tetrahedra form. SRO through NC share the same bond + angle weights (1.65 / 1.35). The order ladder is built by progressively growing the grain (15 → 20 → 26 → 35 Å) and the relaxation budget (250 → 300 → 350 → 400 steps) while tightening ``displacement_sigma`` (0.010 → 0.008 → 0.006 → 0.003). Larger crystalline grain interiors and longer FIRE budgets give the boundary atoms more time to settle into tetrahedral coordination. Larger weights saturate at the same number of detected SiO₄ tetrahedra while distorting boundary atoms past the 0.10 / 18° detector tolerance. The benchmark ladder (rng seed 42, 40 Å cell, 0.10 / 18° detector) walks ≈ 668 (amorphous) → 788 (SRO) → 895 (MRO) → 1022 (LRO) → 1141 (NC) clean SiO₄ tetrahedra out of 1622 Si atoms, a monotonic 41 % → 70 % progression.